Second-order susceptibility from a tight-binding Hamiltonian
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Using a new formalism that modifies a tight-binding Hamiltonian to include interaction with a time-dependent electromagnetic field, we have obtained an analytical expression for the second-order susceptibility. This expression has been used to calculate the energy dependence of X-(2)(omega) for GaAs. The results are in agreement with previous calculations and with available experimental data. [S0163-1829(98)01848-7].